戴启广(Qiguang Dai),博士,1979年7月,出生于安徽省广德县
华东理工大学化学与分子工程学院工业催化研究所
副教授,硕士生导师
办公室:徐汇校区实验8楼214室
E-mail: daiqg@ecust.edu.cn
硕士第一招生专业:工业催化
教育及工作经历:
2018.09-华东理工大学工业催化研究所副教授
2011.10-2018.09华东理工大学工业催化研究所讲师
2009.03-2011.10华东理工大学博士后
2005.09-2009.03华东理工大学工业催化博士
2002.09-2005.07华东理工大学工业催化硕士
1998.09-2002.07安徽工业大学化工工艺学士
研究方向:
稀土、稀土-分子筛杂化纳米材料的可控合成及其在环境催化中的应用,具体围绕以下几个方面开展基础与应用研究:
1. 晶面、形貌可控氧化铈纳米材料合成
2. 结构可控氧化铈-分子筛杂化纳米材料合成
3. 氧化铈基催化剂上CVOCs的低温催化燃烧净化(垃圾焚烧、氯碱)及广谱抗氯VOCs催化剂的开发
4. 传统VOCs低温催化燃烧消除(废气净化、零级空气)
5. 甲烷低温、高温催化燃烧(废气净化、能源利用)
6. 甲烷、长链烷烃、烯烃、芳烃贫氧低温催化氧化(油气储运)、臭氧室温分解(机载臭氧转换器)
7. 难降解高浓度有机废水、低浓度有机废气的液相高级氧化
主持国家自然基金青年项目“疏水性氧化铈基纳米材料的制备及其在含氯有机污染物低温催化净化中的应用”、上海市自然科学基金(面上)“CeO2@ZSM-5分子筛膜复合催化材料的制备及其低温催化消除含氯有机污染物的研究”、高热稳定性、高表面积铈锆固溶体的研发(企业横向项目)和气态氚催化氧化整体式催化剂的研发及其在熔盐反应堆氚监测中的应用(氘代甲烷的催化燃烧,中科院核辐射与核能技术重点实验室开放基金项目)等多个项目。作为主要学术骨干参与了国家重点研发计划“大气污染成因与控制技术研究”试点专项“化工行业典型VOCs催化净化技术的研究及应用示范”,国家科技部863项目“稀土催化氧化关键技术材料及应用”(2011AA03A406),国家科技部863项目专题“稀土/过渡金属/多孔材料催化剂上含氯有机化合物催化消除的研究”(206AA06Z379),多项国家基金委国家自然科学基金项目“Pt基/介孔分子筛催化净化氯代烃类废气研究”(20377012)、“过渡金属氧化物/CeO2纳米催化剂上二恶英类有机化合物催化消除研究”(20977029)、“铈基纳米材料催化剂上氯代有机污染物的低温催化消除”(21277047)和“稀土基催化剂上含氧、含氯挥发性化合物低温催化消除研究”(21477036),军工项目“机载耗氧型惰化系统中催化剂及催化器研究”等10余项项目。先后获得2012年上海市科技进步奖二等奖一项、2015年上海市科技进步奖二等奖一项和2015年教育部科技进步奖二等奖一项,入选首批华东理工大学优秀青年教师培育计划。在国内外学术刊物上发表学术论文43篇(其中SCI、EI收录论文41篇,论文总引用次数为1682次,个人H指数为25);申请专利29篇(包括一项国际专利),其中授权发明专利5项;长期作为多个催化、环境领域国际期刊如Applied Catalysis B: Environmental、Environmental Science & Technology、Catalysis Science & Technology、Catalysis Communications、RSC Advances、Journal of Colloid and Interface Science、Applied Surface Science、CLEAN - Soil, Air, Water、Mendeleev Communications等的审稿人并得到期刊主编们的认可和好评;主编或编著《化学与应用化学专业英语》和《催化剂表征》两本书籍,并主讲《固体催化剂设计与制备》和《固体催化材料》两门催化专业课程。
获奖及荣誉:
获得2018年上海市自然科学奖二等奖(排名第2)
获得2015年教育部科学技术进步奖二等奖(排名第4)
获得2015年上海市科技进步奖二等奖(排名第4)
获得2012年上海市科技进步奖二等奖(排名第5)
发表论文与专著:
[38] Yufeng Gu, Ting Cai, Xiaohui Gao, Hangqi Xia, Wei Sun, Jian Zhao, Qiguang Dai, Xingyi Wang, Catalytic Combustion of Chlorinated aromatics over WOx/CeO2 Catalysts at Low temperature,Applied Catalysis B: Environmental, 2018, https://doi.org/10.1016/j.apcatb.2018.12.055
[37] Qiguang Dai, Zhiyong Zhang, Jiaorong Yan, Jinyan Wu, Grayson Johnson, Wei Sun, Xingyi Wang, Sen Zhang, and Wangcheng Zhan, Phosphate-Functionalized CeO2 Nanosheets for Efficient Catalytic Oxidation of Dichloromethane, Environ. Sci. Technol., 2018,52(22):13430-13437.
[36] Z Zhang, J Huang, H Xia, Qiguang Dai, Y Gu, Y Lao, X Wang, Chlorinated volatile organic compound oxidation over SO42−/Fe2O3 catalysts, Journal of Catalysis, 2018, 360, 277-289.
[35] Z Zhang, H Xia, Qiguang Dai, X Wang, Dichloromethane oxidation over FexZr1-x oxide catalysts,Applied Catalysis A: General 557, 108-118.
[34] Qiguang Dai*, Qin Zhu; Yang Lou; Xingyi Wang*, Role of Brønsted Acid Site during Catalytic Combustion of Methane over PdO/ZSM-5: Dominant or Negligible?, Journal of Catalysis, 357, 2018, 29-40.
[33] Wei Wang, Qin Zhu, Feng Qin, Qiguang Dai*,Xingyi Wang*, Fe doped CeO2 nanosheets as Fenton-like heterogeneous catalysts for degradation of salicylic acid, Chemical Engineering Journal, 333, 2018, 226-239.
[32] Shuxing Bai, Qi Shao, Pengtang Wang, Qiguang Dai, Xingyi Wang, and Xiaoqing Huang*† , Highly Active and Selective Hydrogenation of CO2 to Ethanol by Ordered Pd–Cu Nanoparticles, J. Am. Chem. Soc., 2017, 139 (20),6827-6830.
[31] Yang Lou, Jian Ma, Wende Hu, Qiguang Dai, Li Wang, Wangcheng Zhan, Yanglong Guo, Xiao-Ming Cao, Yun Guo, Peijun Hu, and Guanzhong Lu, Low-temperature methane combustion over Pd/H-ZSM-5: active Pd sites with specific electronic properties modulated by acidic sites of H-ZSM-5, ACS Catal., 2016, 6 (12), 8127-8139.
[30] Tiantian Wang, Qiguang Dai*, Fuwu Yan*, Effect of Acid Sites on Catalytic Destruction of Trichloroethylene over Solid Acid Catalysts, Korean Journal of Chemical Engineering, 2016
[29] Wei Wang, Qin Zhu, Qiguang Dai*, Xingyi Wang, Fe doped CeO2 nanosheets for catalytic oxidation of 1, 2-dichloroethane: Effect of preparation method,Chemical Engineering Journal, 307, 2017, 1037-1046.
[28] Qiguang Dai, Wei Wang, Xingyi Wang, , Guanzhong Lu, Sandwich-structured CeO2@ZSM-5 hybrid composites for catalytic oxidation of 1, 2-dichloroethane: An integrated solution to coking and chlorine poisoning deactivation, Applied Catalysis B: Environmental, 2017, 203, 31-42.
[27] Qiguang Dai,Shuxing Bai,Yang Lou,Xingyi Wang,Yun Guo,Guanzhong Lu, Sandwich-like PdO/CeO2 nanosheet@HZSM-5 membrane hybrid composite for methane combustion: self-redispersion, sintering-resistance and oxygen, water-tolerance, Nanoscale, 2016, 8(18):9621-9628.
[26] Qiguang Dai, Li-Li Yin, Shuxing Bai, Wei Wang, Xingyi Wang, Xue-Qing Gong, Guanzhong Lu, Catalytic total oxidation of 1, 2-dichloroethane over VOx/CeO2 catalysts: Further insights via isotopic tracer techniques, Applied Catalysis B: Environmental, 182 (2016) 598-610.
[25] Shuxing Bai, Qiguang Dai*, Xinxin Chu, Xingyi Wang, Dehydrochlorination of 1,2-dichloroethane over Ba-modified Al2O3 catalysts, RSC Adv., 2016, 6, 52564-52574.
[24] Wei Deng, Qiguang Dai, Yijie Lao, Bingbing Shi, Xingyi Wang, Low temperature catalytic combustion of 1, 2-dichlorobenzene over CeO2-TiO2 mixed oxide catalysts, Applied Catalysis B: Environmental, 181 (2016) 848-861.
[23] Qiguang Dai, Shuxing Bai, Hua Li, Wei Liu, Xingyi Wang, Guanzhong Lu, Catalytic total oxidation of 1, 2-dichloroethane over highly dispersed vanadia supported on CeO2 nanobelts, Applied Catalysis B: Environmental, 168 (2015) 141-155.
[22] Ting Cai, Hao Huang, Wei Deng, Qiguang Dai, Wei Liu, Xingyi Wang, Catalytic combustion of 1, 2-dichlorobenzene at low temperature over Mn-modified Co3O4 catalysts, Applied Catalysis B: Environmental, 166 (2015) 393-405.
[21] Shuxing Bai, Bingbing Shi, Wei Deng, Qiguang Dai*, Xingyi Wang, Catalytic oxidation of 1, 2-dichloroethane over Al2O3-CeO2 catalysts: combined effects of acid and redox properties, RSC Advances, 5 (2015) 48916-48927.
[20] Qiguang Dai, Shuxing Bai, Xingyi Wang, Guanzhong Lu, Facile synthesis of HZSM-5 with controlled crystal morphology and size as efficient catalysts for chlorinated hydrocarbons oxidation and xylene isomerization, Journal of Porous Materials, 21 (2014) 1041-1049.
[19] Hao Huang, Qiguang Dai, Xingyi Wang, Morphology effect of Ru/CeO2 catalysts for the catalytic combustion of chlorobenzene, Applied Catalysis B: Environmental, 158 (2014) 96-105.
[18] Yang Lou, Jian Ma, Xiaoming Cao, Li Wang, Qiguang Dai, Zhenyang Zhao, Yafeng Cai, Wangcheng Zhan, Yanglong Guo, P Hu, Guanzhong Lu, Yun Guo, Promoting Effects of In2O3 on Co3O4 for CO Oxidation: Tuning O2 Activation and CO Adsorption Strength Simultaneously, ACS Catalysis, 4 (2014) 4143-4152.
[17] Yuanjiao Lu, Qiguang Dai, Xingyi Wang, Catalytic combustion of chlorobenzene on modified LaMnO3 catalysts, Catalysis Communications, 54 (2014) 114-117.
[16] Xingyi Wang, Le Ran, Yu Dai, Yuanjiao Lu, Qiguang Dai, Removal of Cl adsorbed on Mn-Ce-La solid solution catalysts during CVOC combustion, Journal of colloid and interface science, 426 (2014) 324-332.
[15] Qiguang Dai, Shuxing Bai, Hua Li, Wei Liu, Xingyi Wang, Guanzhong Lu, Template-free and non-hydrothermal synthesis of CeO2 nanosheets via a facile aqueous-phase precipitation route with catalytic oxidation properties, CrystEngComm, 16 (2014) 9817-9827.
[14] Yang Lou, Xiao-Ming Cao, Jinggang Lan, Li Wang, Qiguang Dai, Yun Guo, Jian Ma, Zhenyang Zhao, Yanglong Guo, P Hu, Guanzhong Lu, Ultralow-temperature CO oxidation on an In2O3-Co3O4 catalyst: a strategy to tune CO adsorption strength and oxygen activation simultaneously, Chemical Communications, 50 (2014) 6835-6838.
[13] Qiguang Dai, Shuxing Bai, Jianwei Wang, Meng Li, Xingyi Wang, Guanzhong Lu, The effect of TiO2 doping on catalytic performances of Ru/CeO2 catalysts during catalytic combustion of chlorobenzene, Applied Catalysis B: Environmental, 142 (2013) 222-233.
[12] Qiguang Dai, Shuxing Bai, Xingyi Wang, Guanzhong Lu, Catalytic combustion of chlorobenzene over Ru-doped ceria catalysts: Mechanism study, Applied Catalysis B: Environmental, 129 (2013) 580-588.
[11] Qiguang Dai, Shuxing Bai, Zhengyi Wang, Xingyi Wang, Guanzhong Lu, Catalytic combustion of chlorobenzene over Ru-doped ceria catalysts, Applied Catalysis B: Environmental, 126 (2012) 64-75.
[10] Qiguang Dai, Hao Huang, Yu Zhu, Wei Deng, Shuxing Bai, Xingyi Wang, Guanzhong Lu, Catalysis oxidation of 1, 2-dichloroethane and ethyl acetate over ceria nanocrystals with well-defined crystal planes, Applied Catalysis B: Environmental, 117 (2012) 360-368.
[9] Yu Dai, Xingyi Wang, Qiguang Dai, Dao Li, Effect of Ce and La on the structure and activity of MnOx catalyst in catalytic combustion of chlorobenzene, Applied Catalysis B: Environmental, 111 (2012) 141-149.
[8] Hongfeng Li, Guanzhong Lu, Qiguang Dai, Yanqin Wang, Yun Guo, Yanglong Guo, Efficient Low-temperature Catalytic Combustion of Trichloroethylene over Flower-like Mesoporous Mn-doped CeO2 Microspheres, Applied Catalysis B: Environmental, 102(2011) 475-483.
[7] Dai Yu, Wang Xingyi, Li Dao, Qiguang Dai, Catalytic Combustion of Chlorobenzene over Mn-Ce-La-O Mixed Oxide Catalysts, Journal of Hazardous Materials, 188 (2011) 132-139.
[6] Meng Wu, Xingyi Wang, Qiguang Dai, Yaoxing Gu, Dao Li, Low temperature Catalytic Combustion of Chlorobenzene over Mn-Ce-O/γ-Al2O3 Mixed Oxides Catalyst, Catalysis Today, 158 (2010) 336-342.
[5] Meng Wu, Xingyi Wang, Qiguang Dai, Dao Li, Catalytic Combustion of Chlorobenzene over Mn-Ce/Al2O3 Catalyst Promoted by Mg, Catalysis Communications, 11 (2010) 1022-1025.
[4] Hongfeng Li, Guanzhong Lu, Qiguang Dai, Yanqin Wang, Yun Guo, Yanglong Guo, Hierarchical Organization and Catalytic Activity of High-Surface-Area Mesoporous Ceria Microspheres Prepared Via Hydrothermal Routes, ACS Appl. Mater. Interfaces, 2 (2010) 838-846.
[3] Qiguang Dai, Xingyi Wang, Guanzhong Lu, Low-temperature catalytic combustion of trichloroethylene over cerium oxide and catalyst deactivation, Applied Catalysis B: Environmental, 81 (2008) 192-202.
[2] Qiguang Dai, Xingyi Wang, Guanzhong Lu, Low-temperature catalytic destruction of chlorinated VOCs over cerium oxide, Catalysis Communications, 8 (2007) 1645-1649.
[1] Qiguang Dai, Xingyi Wang, Guoping Chen, Yi Zheng, Guanzhong Lu, Direct synthesis of Cerium (III)-incorporated SBA-15 mesoporous molecular sieves by two-step synthesis method, Microporous and mesoporous materials, 100 (2007) 268-275.